Puhx
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The Pu+H2 reaction is catalyzed by Pu2O3 and PuHx is produced by the Pu+H2O reaction only at conditions where Pu2O3 formation is kinetically favored. Thermal.
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Based on ab initio calculations within the density-functional theory (DFT)+U theoretical formalism, we systematically study the electronic properties of.
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The solid product expanded in the shape of the Pu sample during reaction and consisted of a PuHx core surrounded by a thick Pu2O3 layer.
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Reaction continues until all Pu is consumed and forms solids with PuHx cores similar to those observed during reaction of O2. H2 is produced if spalled.
exothermic reaction of the cubic solid-solution hydride (PuHx, ≤x≤3) initiates spontaneously upon exposure to air at room temperature.
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Corpus ID: Structural, magnetic, electronic, and elastic properties of face-centered cubic PuHx （x=2, 3） ： GGA （LSDA） ＋ U ＋ SO.
metal sample containing Pu and PuOH results in hydride (PuHx)- catalyzed corrosion of the residual Pu. Kinetics of the first-order.
sThe behavior is further complicated by the possibility of partial hydrogen retention in the cubic PuHx phase. Two possible reactions are described by.
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4 Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing, , China. puhxb@[HOST]
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of the H atoms bond with Pu to precipitate PuHx on the surface of the sample with x ∼ We observe magnetic hysteresis loops below 40 K with magnetic.