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Applied Physics Letters
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Volume 96, Issue 25
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10.1063/1.3456730
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Submitted: 25 April 2010
Accepted: 03 June 2010
Published Online: 21 June 2010
Magnetodielectric effect in EuZrO 3
Appl. Phys. Lett. 96 , 252901 (2010);
https://doi.org/10.1063/1.3456730
T. Kolodiazhnyi K. Fujita L. Wang Y. Zong K. Tanaka Y. Sakka E. Takayama-Muromachi
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Following recent report on antiferromagnetic ordering in EuZrO 3 we performed dielectric measurements of this material as a function of temperature and magnetic field. Dielectric constant of dense EuZrO 3 ceramics is 30.1 at 300 K. It gradually decreases upon cooling without any quantum paraelectric behavior; however, below T N = 4.1 K it shows a pronounced drop that qualitatively resembles that observed in EuTiO 3 . We report that dielectric constant of EuZrO 3 is magnetic field dependent. The magnitude of the magnetodielectric effect in both EuTiO 3 and EuZrO 3 is discussed in the light of the recently proposed coupling of the Eu–O–Eu superexchange interactions with electrons involved in partially covalent Ti(Zr)–O bond.
This work has been supported by Grant-in-Aid for Scientific Research Grant No. 21560025 (T.K.) and Scientific Research on Priority Area Grant No. 22015011 (K.F.) from MEXT Japan.
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