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X-ray pure samples of EuMgSi were synthesized by reactions of the elements in sealed niobium tubes using a high frequency and subsequently a resistance furnace. Powder synchrotron radiation diffraction experiments did not reveal any structural changes down to 4. Two distinct magnetic anomalies around 12 and 14 K can be observed for different samples with dc- and ac-susceptibility, heat capacity and resistivity measurements. Electronic structure calculations in coincidence with the resistivity measurement prove narrow or nearly zero gap-semiconducting behaviour. The calculated band gap energy of 0. In consensus of dc- and ac-susceptibility and neutron powder diffraction a complex combination of antiferromagnetic and ferromagnetic interactions, most likely by super-exchange, is confirmed. These cause two magnetic ordering temperatures, though only one independent crystallographic Eu site in terms of the crystal structure is present in EuMgSi. Niehaus, D. Ryan, R. Flacau, P. Lemoine, D. Chernyshov, V. Svitlyk, E. Cuervo-Reyes, A. Slabon, R. Nesper, I. Schellenberg and R. C , , 3 , DOI: To request permission to reproduce material from this article, please go to the Copyright Clearance Center request page. If you are an author contributing to an RSC publication, you do not need to request permission provided correct acknowledgement is given. If you are the author of this article, you do not need to request permission to reproduce figures and diagrams provided correct acknowledgement is given. Read more about how to correctly acknowledge RSC content. Fetching data from CrossRef. This may take some time to load. Loading related content. Jump to main content. Jump to site search. You do not have JavaScript enabled. Please enable JavaScript to access the full features of the site or access our non-JavaScript page. Issue 27, From the journal: Journal of Materials Chemistry C. Niehaus , a D. Ryan , b R. Flacau , c P. Lemoine , d D. Chernyshov , e V. Svitlyk , e E. Cuervo-Reyes , fg A. Slabon , f R. Nesper , f I. Schellenberg a and R. You have access to this article. Please wait while we load your content Something went wrong. Try again? Cited by. Download options Please wait Article type Paper. Submitted 11 Apr Accepted 06 Jun First published 08 Jun Download Citation. Author version available. Download author version PDF. Request permissions. Social activity. Search articles by author O. This website collects cookies to deliver a better user experience. See how this site uses Cookies. Do not sell my personal data. Veja como este site usa Cookies.

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